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Analysis

This paper explores the use of shaped ultrafast laser pulses to control the behavior of molecules at conical intersections, which are crucial for understanding chemical reactions and energy transfer. The ability to manipulate quantum yield and branching pathways through pulse shaping is a significant advancement in controlling nonadiabatic processes.
Reference

By systematically varying pulse parameters, we demonstrate that both chirp and pulse duration modulate vibrational coherence and alter branching between competing pathways, leading to controlled changes in quantum yield.